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I'll agree with some, every game (I have not played RBY or GSC) has its part with awesome music - really gets me excited and pumped up for the battle or what ever scene is going on. Sort of like preparing for the unexpected.
Overall, I love the music/soundtrack in the Black2/White2 game - pretty much every gym battle (especially with Roxie) and Elite 4.
My favorite themes were the Tin Tower in GSC and the Distortion World in Platinum. Very few songs have made me feel like I was literally in another world but somehow those particular 2 managed to pull it off.
It'd be nice to some day read a post of yours in which you DON'T take the opportunity to go beyond the scope of the question to complain about RSE. It's extremely tedious.