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Nope, it's possible - it's just that legendary Pokemon are usually hard to catch because, well, they're ultra-super-special-Pokemon and hence pose more of a challenge! (I say usually because Palkia/Dialga are exceptions for instance... =/). You already have the status thing going which helps with catching but you just need some more luck with it is all. I will however suggest trying Dusk Balls at night or Net Balls because they have a better catch rate than Ultra Balls for Suicune.
Not much else to discuss here, and if you have any other questions ask in the Help thread sticky. Closed, and good luck with catching it.
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