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I'd have to say Aspertia City by far. It's the first starting town in any Pokemon game where I actually revisit it constantly for the scenery, music, and the atmosphere.
Recently I've been using this current moveset for my (4 HP/252 Sp.Atk/252 Spd) Blastoise:
Water Spout
Ice Beam
Surf
Waterfall
Item: Choice Specs
Note: The two HMs are entirely for the overworld gameplay.
Blastoise can outspeed about half of his opponents I find, so the idea of Water Spout...