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It was the Frontier Brain Anabel if I remember correctly. I actually liked her and the interactions she had with Ash. She was my favorite Frontier Brain actually.
You know the drill lol.
For me the three episodes with Ash vs. Paul at the Sinnoh league are on there and also the episode that had Dawn vs. Zoey in the Grand festival final round is on my list too.
Name says it all :).
For me the two episodes that had Ash's third try to beat Brandon at the Battle Pyramid are definitely on the list. Just curious to see what other people think.