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I did enjoy Gosick's Opening a lot recently, the one ending that sticks out in my head a lot would be a more recent one Gintama Season 5 - Samurai Heart.
Probably my most favourite opening from anime would have to be My Soul, Your Beats from Angel Beats! It's just one of those rare openings which you can't skip. I also enjoyed We Are, and Believe in Wonderland, One Piece's first and second openings and I also enjoyed the Highschool of the Dead opening, which name escapes me.