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Sailormoon was the first I remember watching, although there might've been something else before that. (I vaguely remember Samurai Pizza Cats, but I don't know if I started the series before or after seeing my first Sailormoon episodes.) Yes, I feel old.
As for manga, Pokemon. However, the first series I've read in completion was Wish, followed by Chobits. (I still am a fan of CLAMP.)
My first anime was Ranma 1/2, and the first manga that I read was Sailor Moon (the old Mixx version). I was so into Ranma 1/2 back in the day. I loved Ryoga/P-chan. I thought he was the cutest thing ever. ^_^
My first anime was Voltez V, I think (if that even counts as an anime). Or Akazukin Cha Cha. Oh, or it could have been Yu Yu Hakusho. I don't really remember, but it was definitely one of those.
And I think Naruto was my first manga. I'm pretty sure that wasn't anything before that.
Anime - Nintama Rantarou, back in my home country
Manga - My dad's Golgo 13. I couldn't read kanji back then, so I was basically looking at the "scary looking man" shoot people.