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My favorite OPs are "Moonlight Densetsu" from Sailormoon and "Higurashi no Naku Koro ni" from... Higurashi no Naku Koro ni. C:
I don't usually like EDs though, my favorite is "Tuxedo Mirage" from Sailormoon. :[
edit: oh, and "Unnamed world" from Niju Mensou no Musume
Only a few stand out, although the ones that use clips from episodes are the worst. D:
Anyway, Kibou no Kakera from PPGZ, Hito Toshite Jiku ga Bureteiru from Sayonara Zetsubou Sensei and Motteke! Sailor Fuku from Lucky Star. Don't think I've watched many endings, I usually just skip to the next episode. don't say 'lazy' from K-ON! is an exception.
It usually varies with whatever I'm watching, but I thought ダイアモンド クレバス (Diamond Crevasse) by May'n was pretty good (first ending theme for Macross Frontier). Come to think of it, I liked all the music from Macross Frontier, especially Megumi's stuff (voice of Ranka Lee).
Dragon Soul [Opening for Dragon Ball Kai]
Yeah! Break! Care Break! [Ending for Dragon Ball Kai]
Love For You [22 Op for Detective Conan(I think)]
YUI[Opening for Fullmetal Alchemist: BrotherHood]
USO[Ending for Fullmetal Alchemist: Brotherhood]
Revive[24 OP for Detective Conan]
Mysterious Eyes[7 Op for Detective Conan]
MYSTERIOUS[23 Op for Detective Conan]
Rewrite[4th Opening of Fullmetal Alchemist]