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I think Froslass has the coolest cry. It gives me the chills, and sometimes I look at her pokedex page solely for the purpose of hearing that ghostly-ish cry.
I like Mesprit's cry and......Rotom's....and Dialga's......and I like Gallade's too. Sounds really, real. I also like Cresselia's I just love the way it sounds
Eevee slowed down = Demonic
Glaceon is awesome =
Giratina slowed down = wtf
Hippopotas (slowed down) = Epic
Hippopotas = Cool.
PorygonZ and Cresselia = Great
Luxray is awesome.
Lopunny slowed is uber.
Dialga's is mah favourite (especially from PMD2{ roaring owns}) He's crazy lol. Chatot's cry is just weird and Wigglytuff from PMD2 (YOOM-TAH!!) is funny and makes all kinda crap happen. You know, they never explained how he was so strong he almost blows up the guild every time he gets sad or angry
Okey, okey, I admit that I have played the Gen III and Gen IV games with the sound turned off, BUT, back in Gen II, NO ONE had as great a cry as Electabuzz. It actually had a tune you could listen to constanly without growing bored of it. <3
(This picture is just to prove how awesome it is :D)