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I would have to say CELE-B-R-A-T-E because it had a nice sound to it. But I also like the soundtrack to Pokemon The First Movie and Pokemon the Movie 2000. I like all Pokemon song from the movies.
Personally, the first three I think were all equally great. Unfortunately, I haven't seen the newest three movies(4ever, Mewtwo Returns, Heroes), so I can't really compare all of them, except 'You & Me & Pok?mon'. I got the 'Totally Pok?mon' CD. For anyone who wants to listen to it, go to https://www.pokemon.com (duh) and click the Jukebox link.
Definitely To Know the Unown.
It was the only song who got me to not leave the cinema before I've seen all the ending credits. It suited the movie perfectly, and the girls got nice voices.
But...The Power of One was really beatiful too...