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I have now have got Jigglypuff's level up to 73 , i put lugia to sleep , i got Lugia's health down to a minimum and used alot of ultra balls and i still couldn't catch it.
Just keep trying, it takes a long time to tame lugia but you will succeed eventually. Just keep making it fall asleep and trying to catch it. I used my master ball on it because, as my name suggests, lugia is my favorite.