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Sassy + Latias = No. It hinders one of her most important stats. Calm, Timid, or Modest is the way to go. Can't do much with move sets but I know what natures they need.
Psychic has terrible type coverage...these are both walled by TTar very much, boltbeamer=goodness. Latios can get DD, so if you want a novelty set, use DD and some physical attacks like dragon claw.