I'd like to in Soul Siver, if only so my Pokemon would stop doing cute things when following me and actually act like bad-a**es, but I end up giving up on that since merely WALKING with them increases friendship. For me it's always easier to make them friendly and power up Return.
Since seeing the Rocket Executive in Stadium 2 use Frustration in battle, I've wanted a team of angry Frustration-using Pokemon, but it's so hard to max it out so I end up going the Return route...