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My favorite would definitely have to be Mt. Silver, considering that I go there all the time just to fight Red. XD; Other than Mt. Silver, I guess it would be the Ruins of Alph. :O
National Park, because I like the music and as far as I can remember it's the only place where you get that different sprite for tall grass. Plus, bug catching contests rock (I won one with a L. 18 caterpie against a pinsir and butterfree!).
I also like how the people there advertise for printing out stickers. xD