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Hmm... most Steel-types aren't really all that cute, but I'd have to say that Jirachi and Klink would get my votes, Jirachi especially. With Klink, just look at it. A cute little gear with eyes.
Aron is the cutest I'd say. It's a sort of timid-looking cuteness in a hard exterior. Something about the eyes makes me want it to be in my team every single time.