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Diagla for me, it was soo easy to catch, i caught it in 1 quick ball ( at the beginning of the battle ). I turned my ds off and started again because it was anti climax.
Statistically, Palkia and Dialga would probably be the easiest to catch. You have as much of a chance of catching them as a...chansey, Absol, and Chatot. It would be harder to catch pokemon such as Snorlax, Mantine, and Skarmory.
The easiest for me to catch was... Heatran, took me only a 10 ultra/dusks.
Dialga was quite easy for me, I used a Great Ball to catch it. I got lazy with Cresselia and Master Balled it for a good nature. Mesprit wasn't hard, just took a while cos it liked to run and I hadn't sent my Wobbuffet forward at that point. Quick Balls are my new favourite ball now.
Uxie, Giratina and Palkia. Reason for Uxie is because I got it into low HP and threw an Ultra ball at it and it was caught. Giratina and Palkia were easiest because I used a Master ball. the following week after capturing Giratina I gotten a shiny one on GTS
I voted for Dialga. I hit him to get him in the yellow, threw two Ultra Balls, and that was it. Uxie was easy for me as well, but the other non-roaming one was a pain, I think I eventually just got mad and killed it. xD