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I liked the HGSS tracks, certainly more than FRLG's (which, despite what I've been saying, aren't bad), but I think they could do more. I mean, there were some songs that sounded different- Goldenrod was a good example of this, but if I were to choose between GSC's muzack and HGSS', I'd pick GSC for pretty much every track. I'd love to see another remake of either GSC or RBY so that we could get a Champion track that really nails the intensity that the originals try to present.
If they resorted to orchestrated remixes of RS tracks, I would die, though. That would be the greatest thing ever. They have a lot of room for creativity with the 3DS and I plead them to take advantage of it. So I'm hopin'. I'm gonna keep on hopin'.