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Call me cliché if you will, but since Gen III I've had a fondness for Volt Tackle. The animation admittedly leaves a lot to be desired on some games but I just like the idea of charging at your foe shrouded in so much power. WHAM!
Electric has to be my favourite type, despite my fave Pokémon :P
So far as animation goes, only in R/B/Y did Bubblebeam actually look dangerous, and the same goes for Razor Leaf in G/S/C. The latter has to be my favourite animations in any Pokémon game so far. ^^
Ever since I got the chance to have a Rankurusu/Reuniclus, I've loved Psycho Shock the most. <33
The colors, the sound, the animation.. it's beautiful stuff.
My other favorite is Trick Room. I always imagine the battle field flipping upside down in my head when I use it. XD
I'm torn between Pay Day and Bite honestly. Pay Day because it gets you $300 each time you use it (in SoulSilver anyway, I never paid much attention to the moves before Pearl and SoulSilver >_>;;) And bite because most Pokemon seem pretty hurt by it, so it's a good K.O. for me <3 If any of my Pokemon can learn it I make sure they do and keep it, unless Crunch comes up, that's just as good :3
My favourite move, and has been since it was introduced in Generation III, is Aerial Ace, it looks awesome, it never misses, can deliver a decent amount of damage and is a speedy move.