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I like a ton of'em, but here's a few top ones:
Code Geass R2 - World's End
Shakugan no Shana II - Joint
Murder Princess - Hikari Sasuhou
Naruto Shippuden - Closer
Air - Tori no Uta
I prefer endings since most endings are pretty catchy, but here: Super Driver by Aya Hirano, from The Melancholy of Haruhi Suzumiya 2009, Ringo Mogire Beam! by Kenji Ootsuki (Zan SZS OP) and Ambivalent World by Miyuki Sawashiro <Suruga Monkey Chapter OP of Bakemonogatari>
Melancholy of Haruhi Suzumiya 1st season - Bouken Desho Desho?
Digimon Season 2 (Japanese) - Target
Digimon Season 5 (Japanese) - Hirari
Pokémon Season 5(?) (Japanese) - Ready Go!
Tsubasa Reservoir Chronicles - BLAZE
Tsubasa Reservoir Chronicles - IT'S
Ouran High School Host Club - Sakura Kiss
I'd say, BLEACH OP3, Ichirin No Hana, I love High and Mighty Color's music, and it just fits.
The 1st OP to BLEACH is my second fave OP (OrangeRange are cool too).
Actually, the opening for Negima?! Magister Magi Negima or whatever mental name they called the anime is really cute. I never really noticed it before, but it's awesomely kawaii. (I feel justified in using the term, this being JE and all) As is OHSHC's opening, Sakura Kiss.
I especially like the To Heart OP (Feeling Heart), ONE OP (Eternity), To Heart Remember My Memories OP (Daisuki Dayo) and True Love Stories OVA OP (Sweet Connection).