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Scyther, Exeggcute and Tauros for FRLG - in that order. I've got to say, they made a lot of interesting pokemon for the Safari Zone, but they often didn't get much use, as they were hard to track down.
Chansey. :) The R/S/E safari zone is'nt that great in my opinion, I love the FR/LG one much more. And I love Chansey, as a) I just do, b)Heals people c)I know exactly where to find it. :)
I would definately have to say Dratini, Scyther, Kangaskan, Chansey, and Quagsire because I had a pretty awesome Quagsire on my Platinum version before I screwed my game up and had to restart it.