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Thunderbolt and Shadow Ball. They've helped me throughout the games so much and I daresay Thunderbolt is my most-used move ever.. I taught it to almost every party member that could learn it as a kid. xD;;
But Ice Beam and Flamethrower are high up on the list as well. :)
My favorite in-game is U-Turn. I'm not sure why, just a surprising amount of Pokemon can learn it, and it's a lot of fun. :D Also super effective against those pesky psychic and dark types.
I also like those high power, 100% accuracy moves of course hehe, namely Flamethrower, Psychic, Moonblast, Energy Ball, and Ice Beam, in that order.
Since there are waaay too many cool choices, this is going to be hard. But an attack that usually always ends up on my team and i love using is Ice Beam. Its powerful and its the best way to get rid of the nasty dragons in the Pokemon League. (until Fairy type came along...)