Guess the anime

TOARU MAJUTSU NO INDEX (or RAILGUN S could also work!)
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The name would be Blood+. It seems the mods are cracking down on the some of the posts that aren't meeting the 4 words/25 Characters rule.

Well here's my next guess pic.

Spoiler:
 
Your right it was Black Cat as for your pic one of the most well known imouto characters today.
Kirino from Ore no Imouto ga Konnani Kawaii Wake ga Nai.

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