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Catching Mewtwo with an ultra ball is really tough. I managed it one time after freezing him with Articuno and wasting at least 10+ ultra balls.
But other than Mewtwo, I had a hard time catching Tauros and Scyther. In fact, I actually had 150 pokemon in red at one time, and the only one I was missing was Tauros. I just could not catch him. Scyther's pretty tough, but at least you have the option of buying him at the game center.
Well each different file I have it seems theres always one pokemon harder than the rest, but chansey and zapdos are probably the most consistantly hard to catch.
I'd say the hardest Pokemon to catch is a Feebas. Its way too hard to find ... > >
And other Pokemon aren't hard to catch. By the way, Great Balls work better than Ultra Balls on Legendary Pokemon.
Definately Lugia. I can't count how many attempts I made at trying to catch Lugia.
Raikou, Entei, and Suicune were pretty difficult for me to catch, too. Chasing them around from place to place only for them to run when you finally caught them was always incredibly frustrating.
the hardest non-legendary i say i tauros, it has appeared less times than chansey to me and always runs, well thats for FR/LG on ruby/sapp i believe i would have to say chimecho (tooke me 3 hours to find, while searching in the right place)
Legends are the hardest pokemon to catch because they are different from the normal but it also depends on luck and following the instruction to catch a pokemon easily
I think the hardest for me to catch was Tauros.
Chansey was really easy for me - first time I saw him, I caught him with the first safari ball I had. Luck, I guess.
The dogs are really, really hard to find, but easy to catch.
I think its really hard to catch regice i caught the other 2 with 3 ultra balls and it took my master ball to get her regice is now at lv 77.:laugh: my dream team is ....................................glalie walreign munchlax mime jr. rayquaza banette.