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To me, Sinnoh and Kalos. I liked most of the cast interaction moments in said sagas and in addition to that, are home to two of my fave female companions in the series - Dawn and Serena.
The Sinnoh Saga for sure!
I just loved watching it on CITV and Cartoon network when I was younger.
However I just started rewatching the first seasons of pokemon.
I've watched them all in the last few years. I grew up with the Kanto saga, but I have to gote for Sinnoh. This saga is really awesome! But I do love kanto, jotho and Hoenn too. Not a fan of Univa or Kalos saga...