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Try smashing rocks in: Cianwood City, Dark Cave, Kanto Route 19, Rock Tunnel, Vermillion City, Victory Road (Kanto), and Tohjo Falls cave. Though just be aware that it isn't always a guarantee that you'll find a Heart Scale under the rocks you smash there. You might find other items, wild Pokemon, or nothing.
If you have a Pokemon with Pickup that's over level 51, you can bring it around with you, and it might pick up a Heart Scale then. But that's a low percentage.
There's also the chance to buy one for 1000 points at the Pokéthalon Dome on Wednesdays and Sundays.
But your best bet is to use Rock Smash in those areas I first listed over and over again, and see what you can get that way.
If you have a Pokemon with Pickup that's over level 51, you can bring it around with you, and it might pick up a Heart Scale then. But that's a low percentage.
There's also the chance to buy one for 1000 points at the Pokéthalon Dome on Wednesdays and Sundays.
But your best bet is to use Rock Smash in those areas I first listed over and over again, and see what you can get that way.