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I think it's a tie between Raichu and the Alolan Vulpix and Sandshrew lines. They take some of my fave cute 1st Gen Pokemon and make them even more awesome with their new types (namely Vulpix and Sandshrew lines' Ice typing).
Marowak is another honourable mention, since Ghost/Fire was a typing already made awesome.
Exeggutor is just amazingly simple and ingenious at the same time, lol. Not really what one would imagine a pokemon of grass/dragon typing to look like, but it works somehow.
Alolan Marowak and Alolan Raichu are pretty great! While I haven't used any of the Alolan Forms just yet, I'd definitely say those two are my favourites.